Celtic was strong and tight on server 8 til the merger, boasting 2 websites and a chat that never stopped. They took on, and beat the #1 alliance at the time (BoB), in server 8 and remained an active 100 member alliance until the N1 merger.
But my vote would probably go to DaFallen from server 7, which stayed strong through the N1 merger, and was probably the tightest alliance til Age II came and stole some of their thunder.
150+ servers though, it would be hard to pick the best

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